Zengo is legitimate and, as wallets go, unusually well documented. It was founded in Tel Aviv in 2018, was the first consumer wallet to ship multi-party computation instead of a seed phrase, publishes its security model, runs a bug bounty and has said no Zengo wallet has ever been drained. It is non-custodial: Zengo's server share cannot move funds on its own. Its Trustpilot profile of about 1,100 reviews averaging 4.2 out of 5 is stronger than most wallets', and the company replies to nearly all negative reviews.
What Zengo is not is a licensed financial company. It holds no money transmitter license because it does not need one; the buying and selling inside it is done by MoonPay, which is FinCEN-registered and state-licensed, and MoonPay's rules govern who can buy where. The legitimacy question a careful user should ask is about recovery: because one key share lives on Zengo's servers, restoring a wallet depends on Zengo's service being available and its face-scan recovery working, and Zengo has published a guarantee and an escape mechanism to address that.
Anytime Capital is a U.S. money services business with a storefront in Atlanta and an office in Miami. Its wallet is non-custodial too, its cash account is FDIC-insured, and a question about either is answered by a person at (470) 748-2530.